The Influence of Complex Doping on Kinetics of Decomposition and Thermal Stability of Mg-Based Mechanical Alloys
DOI:
https://doi.org/10.15330/pcss.20.4.406-415Keywords:
mechanical alloy, hydrogen sorption properties, thermal stability, kineticsAbstract
Mechanical alloys (MАs) were synthesized by the method of reactive mechanical alloying. At a hydrogen pressure of 0.1 MPa, with the use of thermal desorption spectroscopy, the thermal stability, the kinetics of hydrogen desorption from the hydride phase MgH2 of the obtained MAs were studied. It has been established that the complex doping by of Fe, Si, Ti, leads to a significant improvement in the of hydrogen desorption from the hydride phase MgH2 of MA synthesized by the RMA. Hydrogen capacity CH of MА after reactive grinding for 20 h. was found to be equal to 5.7 % wt. Due to this alloying, the decrease in the thermodynamic stability of MgH2 is not established. The tested materials showed a high potential as hydrogen storage alloys especially for stationary application.
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[32] M. Bououdina, Z.X. Guo, J. Alloys Comp. 336, 222 (2002) (doi:10.1016/S0925-8388(01)01856-4).
[33] M. Tanniru, D.K. Slattery, F. Ebrahimi, Int. J. Hydrogen Energy 35, 3555 (2010) (doi:10.1016/j.ijhydene. 2010.01.109).
[34] M. Tanniru, D.K. Slattery, F. Ebrahimi, Int. J. Hydrogen Energy 36, 639 (2011) (doi:10.1016/j.ijhydene.2010.09.083).
[35] C. Zhou, Z. Z. Fang, J. Lu, X. Luo, C. Ren, P. Fan, Y. Ren, and X. Zhang, J. Phys. Chem. C118, 11526 (2014) ( doi:10.1021/ jp501306w).
[36] S. Bouaricha, L.P. Dodelet, D.Guay, J.Huot, S.Boily, R.Schulz, J. Alloys Compd. 297, 282 (2000) doi:10.1016/S0925-8388(99)00612-X.
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[38] O.G. Ershova, V.D. Dobrovolsky, O.Yu. Khyzhun, Yu.M. Solonin, Physics and chemistry of solid state 12 (4), 1044 (2011).
[39] John J. Vajo, J. Phys. Chem. B 108, 13977 (2004) (doi:10.1021/jp040060).
[40] M. Polanski, J. Bystrzycki, Int. J. Hydrogen Energy 34, 7692 (2009) (doi:10.1016/jihydene2009.06 002).
[41] D.A. Paskevicius, A. Sheppard, C.J. Chaudhary, C.J. Webb, E. Mac, A. Gray, H.Y. Tian, V.K. Peterson, E. Buckley, J. of Hydrogen Energy 36, 10779 (2011) (doi:10.1016/j.ijhydene.2011.05.132).
[42] Motoki Shimada, Hisashi Tamaki, Eiji Higuchi, J. of Materials and Chemical Engineering Jul. 2(3), 64 (2014).
[43] Anna-Lisa Chaudhary, M. Paskevicius, D.A. Sheppard, J. Alloys Compd. 623, 109 (2015) (doi.org/10.1016/j.jallcom.2014.10.086).
[44] J. Crivello, R.V. Denys, M. Dornheim, M. Felderhoff, D.M. Grant, J. Huot, T.R. Jensen, P.De Jongh, M. Latroche, G.S. Walker, C.J. Webb, V.A. Yartys, Appl. Phys. A 122, 85 (2016) (doi:10.1007/s00339-016-9601-1).
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Published
2019-12-15
How to Cite
Ershova, O., Dobrovolsky, V., & Solonin , Y. (2019). The Influence of Complex Doping on Kinetics of Decomposition and Thermal Stability of Mg-Based Mechanical Alloys. Physics and Chemistry of Solid State, 20(4), 406–415. https://doi.org/10.15330/pcss.20.4.406-415
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